Journal
CHEMICAL COMMUNICATIONS
Volume 54, Issue 36, Pages 4601-4604Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8cc02472c
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Funding
- Ministry of Science and Technology [2016YFA0204100]
- National Natural Science Foundation of China [21672178]
- Thousand Youth Talents Plan
- Fundamental Research Funds for the Central Universities
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The intramolecular C(sp(3))-H/C(sp(2))-H cross-coupling of 1,3-dicarbonyl compounds has been achieved through Cp2Fe-catalyzed electrochemical oxidation. The key to the success of these dehydrogenative cyclization reactions is the selective activation of the acidic -C-H bond of the 1,3-dicarbonyl moiety to generate a carbon-centered radical.
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