Journal
CHEMICAL COMMUNICATIONS
Volume 54, Issue 18, Pages 2186-2199Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7cc09949e
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Funding
- MOE Tier 3 Programme [MOE2014-T3-1-004]
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In this Feature Article, we highlight our recent efforts toward stable open-shell singlet diradicaloids and polyradicaloids. A brief review on the historical works in the area is introduced first, followed by discussion on the fundamental electronic and physical properties of open-shell singlet diradicaloids. Then, the structure-diradical character relationships based on our recently developed diradicaloids are presented. Next, the challenges and solutions toward stable polyradicaloids and 3D -conjugated diradicaloids are discussed. Finally, their preliminary material applications are introduced and a perspective view of the area is given.
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