Journal
CATALYSIS TODAY
Volume 327, Issue -, Pages 154-160Publisher
ELSEVIER
DOI: 10.1016/j.cattod.2018.05.019
Keywords
Formaldehyde; Manganese oxide; K+; Catalytic oxidation; Indoor air
Funding
- National Key Research and Development Program of China [2016YFC0204800]
- National Natural Science Foundation of China (NSFC) [51561165015, N_HKU718/15]
- Research Grants Council (RGC) of Hong Kong [51561165015, N_HKU718/15]
- NSFC [21677179, 21506054]
- Guangdong Special Fund for Science & Technology Development (Hong Kong Technology Cooperation Funding Scheme) [2016A050503022]
- Hong Kong Innovation and Technology Support Program [GHP/025/16GD]
- Innovation Platform Construction of Guangdong and Hong Kong [2017B050504001]
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delta-MnO2 was prepared via a facile in-situ redox reaction and used for catalytic oxidation of HCHO, a major indoor air pollutant. The washing treatment during catalyst preparation could impose great effect on content of K+ and catalytic activity. delta-MnO2 catalyst without washing treatment contains the highest content of K+ ion and exhibits the best catalytic activity among various delta-MnO2 samples. The HCHO removal efficiency keeps at 100% for first 600 min. The delta-MnO2 samples were characterized by advanced technologies including XRD, Raman, XPS, TPR, TPD and in-situ DRIFTS. The XPS results indicates that K+ ions increases the AOS value of Mn and the ratio of surface-adsorbed oxygen over delta-MnO2. The content of K+ ions improves the amount and redox ability of surface mobile oxygen species, enhancing catalytic oxidation of HCHO.
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