Journal
CARBON
Volume 134, Issue -, Pages 366-375Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.carbon.2018.03.080
Keywords
Manganese oxide; Carbon nanotube-web paper; Iron oxide; Carbon fiber; Coaxial fiber-shaped supercapacitor
Funding
- Technology Development Program for Strategic Core Materials - Ministry of Trade, Industry and Energy [10047758]
- Basic Science Research Program through the National Research Foundation of Korea (NRF) - Ministry of Education, Republic of Korea [2012R1A6A1029029, 2014M3A7B4052201, 2015R1A2A2A01008398]
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The fiber-shaped supercapacitor is a promising energy storage device in wearable and portable electronics because of its high flexibility, small size, and light weight. However, most of the reported fiber-shaped supercapacitors have exhibited low capacitance and energy density due to the limited surface area between the two fiber electrodes and operating voltage range. Herein, we successfully developed a coaxial fiber-shaped asymmetric supercapacitor (CFASC) made from MnO2/CNT-web paper as a cathode coupled with Fe2O3/carbon fiber as an anode with a high operating voltage of 2.2 V. The prepared CFASC device showed a high volumetric energy density of 0.43 mWh cm(-3) at a power density of 0.02 W cm(-3), which is comparable to those of previously reported fiber-shaped supercapacitors. Additionally, CFASC exhibited good rate capability, long cycle life, and high volumetric capacitance (0.67 F cm(-3)) with excellent flexibility. The promising performance of CFASC illustrated its potential for portable and wearable energy storage devices. (c) 2018 Elsevier Ltd. All rights reserved.
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