Journal
PHYSICAL REVIEW A
Volume 93, Issue 3, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevA.93.033417
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Funding
- Department of Energy (USA) [DE-FG02-02ER15344]
- National Science Foundation (USA) [CHE-0718610]
- Vice-Chancellor's Postdoctoral Research Fellowship of University of New South Wales, Australia
- U.S. Department of Energy (DOE) [DE-FG02-02ER15344] Funding Source: U.S. Department of Energy (DOE)
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [1464569] Funding Source: National Science Foundation
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Optimal control of quantum systems with complex constrained external fields is one of the longstanding theoretical and numerical challenges at the frontier of quantum control research. Here, we present a theoretical method that can be utilized to optimize the control fields subject to multiple constraints while guaranteeing monotonic convergence towards desired physical objectives. This optimization method is formulated in the frequency domain in line with the current ultrafast pulse shaping technique, providing the possibility for performing quantum optimal control simulations and experiments in a unified fashion. For illustrations, this method is successfully employed to perform multiple constraint spectral-phase-only optimization for maximizing resonant multiphoton transitions with desired pulses.
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