Journal
CHEMCATCHEM
Volume 8, Issue 6, Pages 1028-1032Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cctc.201600037
Keywords
arenes; aromatic substitution; cleavage reactions; photoredox catalysts; radicals
Categories
Funding
- Core Research for Evolutionary Science and Technology (CREST), Japan Science and Technology Agency (JST)
- Japan Society for the Promotion of Science (JSPS)
- Ministry of Education, Culture, Sports, Science and Technology of Japan (MEXT) [26288044, 26620075, 26105708, 26105756, 26870120]
- Grants-in-Aid for Scientific Research [26870120, 26105756, 26288044, 26620075, 26105708, 15H05798] Funding Source: KAKEN
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Novel aromatic substitution reactions of cyanoarenes with 4-alkyl-1,4-dihydropyridines as alkylating reagents in the presence of a catalytic amount of a photoredox catalyst proceed smoothly to give the corresponding alkyl-substituted arenes in good to high yields. The present reaction system realizes a novel C-C bond-forming reaction between two fragments generated from the C-C bond-cleavage reactions of two independent substrates.
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