Journal
PHYSICAL REVIEW B
Volume 93, Issue 15, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.93.155433
Keywords
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Funding
- Department of Science and Technology [SR/S2/LOP-003/2010]
- Council of Scientific and Industrial Research, India [03(1250)/12/EMR-II]
- DST, India [IFA14-MS-25]
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A complex few-layer MoSe2/graphene oxide (GO) heterostructure with strong interlayer coupling was prepared by a facile hydrothermal method. In this strongly coupled heterostructure, we demonstrate a giant enhancement of two-photon absorption that is in stark contrast to the reverse saturable absorption of a weakly coupled MoSe2/GO heterostructure and saturable absorption of isolated MoSe2. Spectroscopic evidence of our study indicates that the optical signatures of isolated MoSe2 and GO domains are significantly modified in the heterostructure, displaying a direct coupling of both domains. Furthermore, our first-principles calculations indicate that strong interlayer coupling between the layers dramatically suppresses the MoSe2 excitonic bands. We envision that our findings provide a powerful tool to explore different optical functionalities as a function of interlayer coupling, which may be essential for the development of device technologies.
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