Journal
RSC ADVANCES
Volume 6, Issue 51, Pages 45495-45502Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6ra09657c
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Funding
- National Natural Science Foundation of China [21173064, 51303043, 21472031, 21503060]
- Zhejiang Provincial Natural Science Foundation of China [LR14B030001]
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To shed light on the scope and limitations of palladium-catalyzed allylic alkylation in the presence of chiral trans-1,2-diaminocyclohexane-derived Fei-Phos as an effective phosphine ligand, the asymmetric palladium-catalysed alkylation of structurally diverse hard/soft nucleophiles, including allylic etherification of alcohols and the allylic alkylation of activated methylene compounds, indoles, and aromatic amines were investigated in this study; the corresponding products with various functional groups were achieved in good yield and with high enantioselectivity (up to 99% ee).
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