Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 57, Issue 37, Pages 12097-12101Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201806674
Keywords
fluorine; N-heterocyclic carbenes; organocatalysis; regioselectivity; trifluoromethylation
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Funding
- Shenzhen STIC [JCYJ20160229205441091]
- Hong Kong RGC [16304115, 16302617, 16311616]
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Described herein is a highly regioselective and efficient N-heterocyclic-carbene-catalyzed gamma-trifluoromethylation of vinylogous enolates. Control experiments and DFT calculations provided important insight into the reaction mechanism.
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