Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 57, Issue 32, Pages 10123-10126Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201804299
Keywords
2D membranes; carbon nitride; energy conversion; ion transport; nanoporous membranes
Categories
Funding
- Alexander von Humboldt Foundation
- Max Planck Society
- National Key Research and Development Program of China [2017YFA0206904, 2017YFA0206900]
- National Natural Science Foundation [21625303, 51673206, 21434003, 91427303]
- Key Research Program of the Chinese Academy of Sciences [KJZD-EW-M03]
- Frontier Science Key Projects of CAS [QYZDY-SSW-SLH014]
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Ions transport through confined space with characteristic dimensions comparable to the Debye length has many applications, for example, in water desalination, dialysis, and energy conversion. However, existing 2D/3D smart porous membranes for ions transport and further applications are fragile, thermolabile, and/or difficult to scale up, limiting their practical applicability. Now, polymeric carbon nitride alternatively allows the creation of an ultrathin free-standing carbon nitride membrane (UFSCNM), which can be fabricated by simple CVD polymerization and exhibits excellent nanofluidic ion-transport properties. The surface-charge-governed ion transport also endows such UFSCNMs with the function of converting salinity gradients into electric energy. With advantages of low cost, facile fabrication, and the ease of scale up while supporting high ionic currents, UFSCNM can be considered as an alternative for energy conversion systems and new ionic devices.
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