Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 57, Issue 35, Pages 11278-11282Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201805632
Keywords
automation; continuous flow; fluorescence quenching experiments; photoredox catalysis; Stern-Volmer
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Funding
- VIDI grant (SensPhotoFlow) [14150]
- Marie Curie ITN Grant (Photo4Future) [641861]
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Herein, we report the first fully automated continuous-flow platform for fluorescence quenching studies and Stern-Volmer analysis. All the components of the platform were automated and controlled by a self-written Python script. A user-friendly software allows even inexperienced operators to perform automated screening of novel quenchers or Stern-Volmer analysis, thus accelerating and facilitating both reaction discovery and mechanistic studies. The operational simplicity of our system affords a time and labor reduction over batch methods while increasing the accuracy and reproducibility of the data produced. Finally, the applicability of our platform is elucidated through relevant case studies.
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