Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 57, Issue 9, Pages 2296-2306Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201710377
Keywords
C-H activation; catalysis; methane; palladium; rhodium; turnover
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Funding
- Alexander von Humboldt Foundation
- Deutsche Forschungsgemeinschaft (Leibniz Award)
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C-H activation reactions with high catalyst turnover numbers are still very rare in the literature and 10 mol% is a common catalyst loading in this field. We offer a representative overview of efficient C-H activation catalysis to highlight this neglected aspect of catalysis development and inspire future effort towards more efficient C-H activation. Examples ranging from palladium catalysis, Cp*Rh-III- and Cp*Co-III-catalysis, the C-H borylation and silylation to methane C-H activation are presented. In these reactions, up to tens of thousands of catalyst turnovers have been observed.
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