4.8 Article

Thermal Imaging with Plasmon Resonance Enhanced HgTe Colloidal Quantum Dot Photovoltaic Devices

Journal

ACS NANO
Volume 12, Issue 7, Pages 7362-7370

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsnano.8b03871

Keywords

HgTe CQDs; thermal imaging; plasmon resonance; photovoltaic devices; midwave infrared

Funding

  1. ARO [W911NF-15-1-0110]
  2. University of Chicago Materials Research Science and Engineering Center - National Science Foundation [DMR-1420709]

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Thermal imaging in the midwave infrared plays an important role for numerous applications. The key functionality is imaging devices in the atmospheric window between 3 and 5 mu m, where disturbance from fog, dust, and other atmospheric influence could be avoided. Here, we demonstrate sensitive thermal imaging with HgTe colloidal quantum dot (CQD) photovoltaic detectors by integrating the HgTe CQDs with plasmonic structures. The responsivity at 5 mu m is enhanced 2- to 3-fold over a wide range of operating temperatures from 295 to 85 K. A detectivity of 4 x 10(11) Jones is achieved at cryogenic temperature. The noise equivalent temperature difference is 14 mK at an acquisition rate of 1 kHz for a 200 mu m pixel. Thermal images are captured with a single-pixel scanning imaging system.

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