4.8 Article

A Thermal Diode Based on Nanoscale Thermal Radiation

Journal

ACS NANO
Volume 12, Issue 6, Pages 5774-5779

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsnano.8b01645

Keywords

thermal rectification; thermal diode; near-field radiative heat transfer; vanadium dioxide; nanoscale heat transfer

Funding

  1. Army Research Office [W911NF-16-1-0195, W911NF-18-1-0004]
  2. DOE-BES [DE-SC0004871]
  3. National Science Foundation [CBET 1509691]
  4. U.S. Department of Energy (DOE) [DE-SC0004871] Funding Source: U.S. Department of Energy (DOE)

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In this work we demonstrate thermal rectification at the nanoscale between doped Si and VO2 surfaces. Specifically, we show that the metal-insulator transition of VO2 makes it possible to achieve large differences in the heat flow between Si and VO2 when the direction of the temperature gradient is reversed. We further show that this rectification increases at nanoscale separations, with a maximum rectification coefficient exceeding 50% at 140 nm gaps and a temperature difference of 70 K. Our modeling indicates that this high rectification coefficient arises due to broadband enhancement of heat transfer between metallic VO2 and doped Si surfaces, as compared to narrower-band exchange that occurs when VO2 is in its insulating state. This work demonstrates the feasibility of accomplishing near-field-based rectification of heat, which is a key component for creating nanoscale radiation-based information processing devices and thermal management approaches.

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