Journal
ACS APPLIED MATERIALS & INTERFACES
Volume 11, Issue 3, Pages 2662-2669Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsami.8b03345
Keywords
full-carbon material; graphdiyne; NiFe LDH; electrocatalyst; oxygen evolution
Funding
- National Natural Science Foundation of China [21771114]
- Natural Science Foundation of Tianjin [17JCYBJC40900]
- Thousand Youth Talents Plan of China
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Graphdiyne (GDY), a novel two-dimensional full carbon material, has attracted lots of attention because of its high conjugated system comprising sp(2) and sp-hybridized carbons. The distinctive structure characteristics endow it unique electronic structure, uniform distributed pores and excellent chemical stability. A novel GDY-supported NiFe layered double hydroxide (LDH) composite was successfully prepared for the first time. By taking advantage of the increased surface active areas and improved conductivity, the designed hierarchical GDY@NiFe composite exhibits outstanding catalytic activity that only required a small overpotential about 260 mV to achieve the current density of 10 mA cm(-2). The nanocomposite shows excellent durability in alkaline medium implying a superior OER electrocatalytic activity. It is anticipated that the as-prepared GDY@NiFe composite electrocatalyst provide new insights in designing graphdiyne-supported electrocatalyst materials for oxygen evolution application.
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