Journal
CHEMCATCHEM
Volume 8, Issue 14, Pages 2340-2344Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cctc.201600186
Keywords
hydrogen; iron; photocatalysis; reduction; water splitting
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Funding
- National Science Foundation of China [21376222, 121361130021, 21372091]
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In situ generated iron-based Knolker complexes were found to be efficient catalysts in a fully non-noble metal Cu-Fe photocatalytic water reduction system. These mononuclear iron catalysts were able to generate hydrogen up to 15 times faster than previously reported [Fe-3(CO)(12)]. A reductive quenching mechanism was shown to operate by fluorescence experiments.
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