Controlled Assembly of Graphene-Based Aerogels

Graphene aerogels are obtained from graphene sheets through wet chemical assembly or vapor phase chemical growth. They have a three dimensional graphene architecture that has an interconnected network with a high specific surface area, good electric conductivity and other physicochemical properties and thus has important applications in electrochemical energy storage, adsorption, catalysis and sensing. In this review, we will highlight the assembly strategies and structural designs used to introduce the controlled assembly of the graphene sheets in graphene aerogel materials, such as graphene oxide-, reduced graphene oxide-, CVD-grown graphene and composite graphene aerogels. The current challenges and future development of the grapheme aerogels are also discussed.