Journal
ACS ENERGY LETTERS
Volume 3, Issue 1, Pages 54-62Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsenergylett.7b00926
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Funding
- Florida State University through the Energy and Materials Initiative
- National Science Foundation (NSF) [DMR-1709116]
- Florida State University through the GAP Commercialization Grant Program
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Organometal halide perovskites have recently emerged as a highly promising class of functional materials for a variety of applications. The exceptional structural tunability enables these materials to possess three- (3D), two- (2D), one- (1D), and zero-dimensional (OD) structures at the molecular level. Remarkable progress has been realized in the research of perovskites in recent years, focusing mainly on 3D and 2D structures but leaving low dimensional 1D and OD structures significantly underexplored. Here we offer our perspective on the most exciting developments in the low-dimensional organometal halide perovskites. Due to the strong quantum confinement and site isolation, 1D and OD perovskites exhibit remarkable and useful properties that are significantly different from those of 3D and 2D perovskites. The excitement about the recent developments lies not only in the specific achievements but also in what these materials represent in terms of a new paradigm in materials design.
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