Journal
EUROPEAN POLYMER JOURNAL
Volume 62, Issue -, Pages 247-272Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.eurpolymj.2014.07.008
Keywords
Thiolactone chemistry; One-pot multi-step click chemistry; Functionalized polymers; Amine-thiol-ene conjugation
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Funding
- Ghent University
- Belgian program on Interuniversity Attraction Poles [P7/05]
- European Science Foundation Precision Polymer Materials (P2M) program
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One-pot multi-step reactions based on thiolactone chemistry emerged as a powerful tool to prepare tailor-made, multi-functionalized polymer architectures in a one-pot and elegant manner. This feature article highlights the most important features of this approach, demonstrated in various reactive systems including (bio-based) linear polymers, heterotelechelic polymers, polymeric networks and heterogeneous supports. This overview clearly reveals its remarkable versatility involving modular synthesis and double modification of polymers: thiolactones can be opened by a wide variety of functional amines and the released thiol can react with thiol 'scavengers' of choice. (C) 2014 Elsevier Ltd. All rights reserved.
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