Journal
JOURNAL OF MATERIALS CHEMISTRY C
Volume 5, Issue 6, Pages 1494-1500Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6tc05037a
Keywords
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Funding
- Natural Science Foundation of China [61421002, 61106040, 61605024, 61475030]
- Program for New Century Excellent Talents in University [NCET-13-0092]
- State Key Laboratory of Electronic Thin Film and Integrated Device Program [KFJJ201408]
- Central University Basic Scientific Research Business Expenses [ZYGX2015Z001]
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van der Waals heterostructures built from two-dimensional (2D) materials have attracted wide attention because of their fascinating electrical and optoelectronic properties. Here, we report a highly responsive and broadband photodetector based on WS2-graphene van der Waals epitaxial heterostructures, which were fabricated by directly growing single crystalline few layer WS2 nanosheets on a polycrystalline graphene film. Upon light illumination, the current apparently reduces because of the transfer of photogenerated electrons from WS2 into the underlying p-type graphene and a photo-gating effect induced by the remaining holes, which is in stark contrast to ordinary semiconducting photoconductors. Thanks to the strong and broadband absorption of WS2, the WS2-graphene heterostructure photodetector exhibits a high responsivity with a maximum of 950 A W-1 at 405 nm and a wide spectrum response ranging from 340 to 680 nm. The high performance can be attributed to the internal built-in electric field at the WS2-graphene interface, which leads to the efficient separation of photogenerated electron-hole pairs. The WS2-graphene heterostructure photodetector may have potential applications in low cost, broadband, and flexible optoelectronics.
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