Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 5, Issue 5, Pages 1957-1961Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6ta09908d
Keywords
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Funding
- Zewail City of Science and Technology
- Egypt Science and Technology Development Fund (STDF) [6125]
- Center for Materials Science
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A heterogeneous catalyst for the proton reduction reaction was constructed through immobilization of cobaloxime, in a microporous solid, atop unmodified graphene sheets through a one-pot reaction. This approach afforded a true heterogeneous catalyst to circumvent the known poor stability of cobaloximes in aqueous solutions. The composite demonstrated significant electrochemical activity and ability to reload the Co ions and with enhanced activity toward proton reduction (an onset of similar to-11 mV and a current density of 9 mA cm (2) at-0.88 V vs. RHE).
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