Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 5, Issue 17, Pages 7801-7805Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7ta01578j
Keywords
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Funding
- Addy/ISN North American Low Carbon Emission Energy Self-Sufficiency Fund at Princeton University
- NSF-DGE [1148900]
- PRISM Imaging and Analysis Center
- NSF-DMR [1420541]
- Division Of Graduate Education
- Direct For Education and Human Resources [1148900] Funding Source: National Science Foundation
- Division Of Materials Research
- Direct For Mathematical & Physical Scien [1420541] Funding Source: National Science Foundation
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Efficient large scale electrochemical energy storage systems, such as those based on multivalent ions, are a prerequisite for the realization of intermittent renewable energy sources. From the perspectives of both cost and environmental concerns, it is of critical importance that components of these systems are synthesized using sustainable chemical processes starting from their initial conception. Herein, we report on a fluorinated dialkoxide-based magnesium-ion electrolyte that is synthesized through an atom-efficient and scalable process without the use of any metal alkyls. The electrolyte composition results in high solution conductivity (4.77 mS cm(-1) at 26.3 degrees C), low overpotentials, ca. 100% coulombic efficiency for electrodeposition/dissolution, and good performance in full battery cells using Chevrel phase Mo6S8.
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