Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 5, Issue 40, Pages 21189-21195Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7ta06658a
Keywords
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Funding
- US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-SC0010596]
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The combined use of porphyrins and fluorides to fabricate pillared coordination sheets is presented. Multiple features, such as coordinatively unsaturated metal sites, an optimal pore space, and a fluoride-decorated internal surface, make the new materials ideal adsorbents with high capacity and affinity for carbon dioxide. In addition, the new materials are shown to be suitable single-source precursors to afford fluorine-doped graphene analogues for application in oxygen reduction reaction electrodes.
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