Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 5, Issue 47, Pages 24965-24971Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7ta08441b
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Funding
- National Research Foundation of Korea [NRF-2016R1A2B3013825, NRF-2017R1D1A1B03035441]
- KU-KIST research fund
- National Research Foundation of Korea [2016R1A2B3013825] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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In this work, we demonstrate that the incorporation of MoS2 nanosheets with Pd nanodots is a promising way for promoting the visible-light-induced Suzuki-Miyaura C-C coupling reaction. The MoS2 nanosheets decorated with Pd nanodots showed very high photocatalytic activity. The turnover frequency for the biphenyl product was >1600 h(-1) even under sunlight illumination at room temperature. Mechanistic studies show that the high catalytic activity originated from the efficient electron-hole pair generation mechanism of MoS2 under visible-light illumination instead of purely thermal effects.
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