4.7 Article

Coupling multiphase-Fe and hierarchical N-doped graphitic carbon as trifunctional electrocatalysts by supramolecular preorganization of precursors

Journal

CHEMICAL COMMUNICATIONS
Volume 53, Issue 12, Pages 2044-2047

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cc09442b

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Funding

  1. National Natural Science Foundation of China [91333110, 21675022]
  2. Natural Science Foundation of Jiangsu Province [BK20160028]
  3. Fundamental Research Funds for the Central Universities

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A hydrogen bond-driven supramolecular strategy to synthesize multiphase-Fe anchoring on hierarchical N-doped graphitic carbon was proposed. As a result, the as-obtained catalysts showed unusual trifunctional activities in the oxygen reduction reaction, oxygen evolution reaction and hydrogen evolution reaction, even surpassing noble-metal catalysts such as Pt/C and RuO2.

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