Journal
ACS APPLIED MATERIALS & INTERFACES
Volume 9, Issue 9, Pages 8113-8120Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsami.6b15710
Keywords
hole-blocking layer-free; grain size; perovskite solar cell; blockage effect; RIM infiltration; recyclability
Funding
- Global Frontier R&D Program on Center for Multiscale Energy System -National Research Foundation under the Ministry of Education, Science and Technology, Korea [2011-0031573, NRF-2014M3A6A7060583]
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There remains tremendous interest in perovskite solar cells (PSCs) in the solar energy field; the certified power conversion efficiency (PCE) now exceeds 20%. Along with research focused on enhancing PCE, studies are also underway concerning PSC commercialization. It is crucial to simplify the fabrication process and reduce the production cost to facilitate commercialization. Herein, we successfully fabricated highly efficient hole-blocking layer (HBL)-free PSCs through vigorously interrupting penetration of hole-transport material (HTM) into fluorine-doped tin oxide by a large grain based-CH3NH3PbI3 (MAPbI(3)) film, thereby obtaining a PCE of 18.20%. Our results advance the commercialization of PSCs via a simple fabrication system and a low-cost approach in respect of mass production and recyclability.
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