Journal
CHEMICAL PHYSICS LETTERS
Volume 672, Issue -, Pages 26-30Publisher
ELSEVIER
DOI: 10.1016/j.cplett.2017.01.046
Keywords
Boron; g-C3N4; Doping; Electrocatalytic reduction; p-nitrophenol
Funding
- National Natural Science Foundations of China [21306067, 21676129]
- Graduate Innovation Fund of Jiangsu Province [SJLX16_0433]
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Herein, we rationally designed 3D carbon nitride hierarchical architecture with an interconnected network of graphene-analogue nanosheets and doped with boron through co-condensation strategy. XPS spectra confirmed the incorporation of boron atoms in the polymeric g-C3N4, while X-ray diffraction and IR indicated the characteristic structural properties of pristine g-C3N4 and boron-doped g-C3N4 (B-x-GCN). The B-x-GCN shows promising electrocatalytic activity and stability in the reduction of pnitrophenol according to cyclic voltammograms analysis. Additionally, the use of this metal-free, organic, semiconducting polymer as an electrocatalyst would open wide application of hybrid carbon nitride materials from both point view of economy and environment.(C) 2017 Elsevier B.V. All rights reserved.
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