Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 56, Issue 13, Pages 3526-3530Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201611785
Keywords
metal-organic frameworks (MOFs); nanosheets; photovoltaics; porphyrins; zinc
Categories
Funding
- JST-PRESTO Hyper-nano-space design toward Innovative Functionality
- JST-CREST Development of Atomic or Molecular Two-Dimensional Functional Films and Creation of Fundamental Technologies for Their Applications
- JSPS KAKENHI [JP25107003, JP26620039, JP26220801, JP26708005, JP15H00862, JP16H00900, JP16H00957]
- Hong Kong Research Grants Council [HKBU 12302114]
- Areas of Excellence Scheme of HKSAR [AoE/P-03/08]
- National Natural Science Foundation of China [51573151, 91333206]
- Science, Technology, and Innovation Committee of Shenzhen Municipality [JCYJ20140419130507116]
- Hong Kong Baptist University [FRG2/13-14/083]
- Hong Kong Polytechnic University
- Grants-in-Aid for Scientific Research [16H00957, 15H00862, 26708005, 26220801, 25107003, 26110505, 15K21722, 16H00900, 26620039] Funding Source: KAKEN
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New bis(dipyrrinato) zinc(II) complex micro- and nanosheets containing zinc(II) porphyrin (N2) are synthesized. A liquid/liquid interface method between dipyrrin porphyrin ligand L2 and zinc acetate produces N2 with a large domain size. N2 can be layered quantitatively onto a flat substrate by a modified Langmuir-Schafer method. N2 deposited on a SnO2 electrode functions as a photoanode for a photoelectric conversion system. The photoresponse of N2 covers the whole visible wavelength range (400-650 nm), with a maximum quantum efficiency of more than twice that of a bis(dipyrrinato) zinc(II) complex nanosheet without porphyrin.
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