Journal
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
Volume 5, Issue 3, Pages 2098-2108Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acssuschemeng.6b01936
Keywords
Phenol steam reforming; H-2 production; Carbon nanotubes; Ni/Fe; Nanocatalysts; S/C
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Funding
- Natural Science Foundation of China [51674262]
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The development of cost and environmentally efficient catalysts is essential to transferring phenolic compounds to valuable fuels and chemicals. Various nanocatalysts with different amounts of Ni/Fe have been employed in the steam reforming of phenol, which showed high performance in terms of activity and stability. The conversion and hydrogen yield of phenol reforming over Ni/Fe-catalysts can reach 87% and 81%, respectively. The catalyst can keep its high reactivity for more than 200 h at the steam to carbon ratio (S/C) of 13.3, which is much higher than the previous report of 13 h. Using the newly developed Ni/Fe-catalysts in this research, the hydrogen-rich syngas or carbon nanotube (CNT) could be selectively produced via simply tuning the S/C ratio. The influence of the Ni/Fe ratio and S/C ratio on the steam reforming performance was investigated.
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