Journal
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
Volume 5, Issue 11, Pages 9651-9656Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acssuschemeng.7b02845
Keywords
Artificial photosynthesis; Electron microscopy; Heterogeneous catalysis; Oxygen evolution; Ruthenium; Water oxidation
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Funding
- Swedish Research Council [621-2013-4872, 621-2013-4868]
- Stiftelsen Olle Engkvist Byggmastare
- Knut and Alice Wallenberg Foundation
- Carl Trygger Foundation
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Herein we report the synthesis of mesoporous ruthenium oxide (MP-RuO2) using a template-based approach. The catalytic efficiency of the prepared MP-RuO2 was compared to commercially available ruthenium oxide nanoparticles (C-RuO2) as heterogeneous catalysts for water oxidation. The results demonstrated superior performance of MP-RuO2 for oxygen evolution compared to the C-RuO2 with respect to recyclability, amount of generated oxygen, and stability over several catalytic runs.
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