Journal
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
Volume 5, Issue 5, Pages 4050-4055Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acssuschemeng.7b00031
Keywords
Magnetic composites; Porous organic polymers; Azo coupling reaction; Dyes removal; Water treatment; Dye separation
Categories
Funding
- National Natural Science Foundation of China [21175102, 21205090, 21575107]
- National Basic Research Program of China (973 Program) [2013CB933900]
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Herein, magnetic porous organic polymers composites (MOPs) with abundant free phenolic hydroxyl group were synthesized via a simple and green azo coupling reaction under mild conditions in water. Remarkably, Fe3O4@SiO2 nanoparticles were encapsulated in the disordering porous organic polymers during the coupling reaction. The prepared MOPs possessed excellent stability, high special surface areas, controllable magnetism, and high adsorption capacity (1153 mg g(-1)) toward cationic dye methylene blue. Moreover, the MOPs could be easily and rapidly recovered from the solution by using a magnet due to their superparamagnetic property and could be reused at least 5 times without decreasing the adsorption capacity, demonstrating a potential application in pollutants removal.
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