Journal
ACS APPLIED MATERIALS & INTERFACES
Volume 9, Issue 13, Pages 11819-11827Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsami.7b01229
Keywords
dog noses; crumpled graphene nanosheets; supramolecular modification; lyophilization; NO2 sensors
Funding
- National Natural Science Foundation of China [51373005, 51673007]
- National Key Basic Research Program of China [2014CB931800]
- Program for New Century Excellent Talents in University [NCET-10-0035]
- Fundamental Research Funds for the Central Universities
- Leading Talents of Guangdong Province Program
- Program for Changjiang Scholars and Innovative Research Team in University [IRT13064]
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It is well-established that the structures dominate the properties. Inspired by the highly :contorted and crumpled maxilloturbinate inside dog nose, herein an artificial nanostructure, i.e., 51) crumpled graphene4msed nanosheets, is reported with the simple fabrication,:cletalled characterizations, and efficient gs-sensing applications. A facile supramblecular noncovalentasSembly is introduced to modify graphene with functional molecules, followed with a lyophilization process to,massively transform 2D- plane graphene-based nanosheets to 3D crumpled structure:: The detailed morphological characterizations reveal that: the bioinspired nanosheets exhibit full, consistency with maxilloturbinate. The fabricated 3D crumpled graphene-based sensors exhibit ultrahigh response (R-a/R-g = 3.8) toward 10 ppm of NO2, which is mainly attributed to the specific maxilloturbinatemimic structure. The sensors also exhibit' excellent selectivity and sensing 'linearity, reliable repeatability, and stability. Interestingly, it is observed that only 4 mg of graphene oxide (GO) raw materials can produce more than 1000 gas sensors, which provides a new insight for developing novel 3D biomimetic materials in large-scale,gas sensor production.
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