Journal
COMPOSITE STRUCTURES
Volume 165, Issue -, Pages 91-98Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.compstruct.2017.01.011
Keywords
Diffusion-induced stresses; Graphene-based composite electrode; Graphene platelets; Stoney formula
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Funding
- National Natural Science Foundation of China [11621062, 11532001, 11402310]
- Fundamental Research Funds for the Central Universities [2016XZZX001-05, 15CX08004A]
- Foundation for Outstanding Young Scientist in Shandong Province [BS2014CL022]
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The diffusion-induced stresses in a bilayer electrode composed of a current collector and a composite active plate of lithium-ion battery are evaluated analytically. The active plate of the bilayer electrode is reinforced by graphene platelets (GPLs), with the corresponding material properties predicted by the combination of the well-established Halpin-Tsai model and the rule of mixture. The diffusion-induced stresses and curvature of the bilayer electrode under either galvanostatic or potentiostatic charging operation are derived. In addition, modified Stoney formulas for the bilayer electrode are developed for the two charging operations. A parametric study is conducted through numerical examples, with a particular focus on the reinforcing effect of GPLs on the stresses and deformation in the bilayer electrode. The size effects of GPLs, including width, length and thickness, on the stresses and deformation are also discussed. (C) 2017 Elsevier Ltd. All rights reserved.
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