Journal
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
Volume 2015, Issue 20, Pages 4320-4324Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.201500623
Keywords
Organocatalysis; Michael addition; Domino reactions; Cycloaddition; Nitro compounds
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Funding
- Ministry of Education, Culture, Sports, Science and Technology (MEXT), Japan [23105010]
- Grants-in-Aid for Scientific Research [14J03546, 25620074] Funding Source: KAKEN
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The enantioselective domino Michael/Henry reaction of nitroalkenes with succinaldehyde was found to proceed efficiently upon using diphenylprolinol silyl ether as the organocatalyst. The reaction affords cis-disubstituted nitropen-tenes with excellent diastereoselectivities and enantioselectivities after treatment of the Michael product with Ac2O and pyridine.
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