Journal
CHEMICAL SOCIETY REVIEWS
Volume 46, Issue 8, Pages 2272-2305Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cs00935b
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Funding
- Natural Science Foundation of China [21502080, 21202073, 21290180, 21272097, 21372104, 21472077]
- 111 Program of MOE
- MOST [2012ZX 09201101-003]
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1,2-Carbon atom rearrangement has been broadly applied as a guiding strategy in complex molecule assembly. As it entails the carbon-carbon or carbon-heteroatom bond migration between two vicinal atoms, this type of reaction is capable of generating structural complexity through a molecular skeletal reorganization. This review will focus on recent employment of this strategy in the total synthesis of natural products, highlighting the exceptional utility of such synthetic methodologies in the construction of intricate carbocycles, heterocycles or structurally complex motifs from synthetically more accessible precursors.
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