Journal
CHEMSUSCHEM
Volume 10, Issue 9, Pages 1898-1903Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201700245
Keywords
carbon; co(2) fixation; doping; heterogeneous catalysis; metal-organic frameworks
Funding
- 973 program [2014CB931803]
- NSFC [21371162, 21673213, 21521001]
- State Key Lab of Materials-Oriented Chemical Engineering [KL15-02]
- Recruitment Program of Global Youth Experts
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The types and quantities of active sites play a critical role in catalysis. Herein, ZnO nanoparticles encapsulated into N-doped porous carbon has been rationally prepared by the pyrolysis of a metal-organic framework (MOF) followed by a moderate oxidation treatment. The resulting catalyst exhibits excellent activity, selectivity, and recyclability in the CO2 cycloaddtion reactions with epoxides owing to the synergy of multiple sites inherited from the MOF and generated by the oxidation process.
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