Journal
CHEMICAL COMMUNICATIONS
Volume 53, Issue 31, Pages 4354-4357Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7cc01707c
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Funding
- National Natural Science Foundation of China [21390400, 21520102003, 21272180, 21302148]
- Hubei Province Natural Science Foundation of China [2013CFA081]
- Research Fund for the Doctoral Program of Higher Education of China [20120141130002]
- Ministry of Science and Technology of China [2012YQ120060]
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Pd/Cu catalyzed oxidative dual C-H bond activation/carbonylation still remains a great challenge due to the generation of by-products via C-C bond formation. Herein we developed a straightforward Pd/Cu-catalyzed oxidative dual C-H bond carbonylation process to access biologically and pharmaceutically important fluorazones from easily available N-aryl pyrroles and CO. A wide range of functional groups were well tolerated in this transformation, and O-2 could be utilized as the only terminal oxidant to promote the oxidative carbonylation process.
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