Journal
ACS MACRO LETTERS
Volume 6, Issue 12, Pages 1352-1356Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsmacrolett.7b00872
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Funding
- National Basic Research Program of China (973 Program) [2013CB834701]
- National Science Foundation of China [21490570, 21490574]
- Research Grants Council of Hong Kong [6308116, 6303815, 6305014, C2014-1567, A-HKUST605/16]
- Nissan Chemical Industries, Ltd.
- Innovation and Technology Commission [ITCRD/17-9]
- University Grants Committee of Hong Kong [AoE/P-03/08]
- Guangdong Innovative Research Team Program [201101C0105067115]
- Shenzhen Peacock Plan
- Science and Technology Plan of Shenzhen [JCY20160229205601482]
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Here we reported a versatile and multicomponent polymerization (MCP) approach that enabled the synthesis of functional poly(propargyl imine)s with well-defined structures and high molecular weight (M-w up to 38 200) in excellent yields (up to 93%) from readily accessible monomers of dibromoarenes, isonitriles, and diynes. This MCP had the advantages of simple operation, wide substrate scope, and mild reaction conditions. The resulting polymers possessed good solubility and showed high thermal stability and refractive indices. The tetraphenylethene-containing polymer displayed a phenomenon of aggregation-induced emission and could respond to various acidic vapors.
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