Journal
CHEMISTRY LETTERS
Volume 46, Issue 6, Pages 808-810Publisher
CHEMICAL SOC JAPAN
DOI: 10.1246/cl.170166
Keywords
Dehydrogenation; Iridium catalyst; Alcohol
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Funding
- JSPS KAKENHI Grant [JP16H01018]
- Asahi Glass Foundation
- Research Foundation for the Electrotechnology of Chubu
- [26288047]
- Grants-in-Aid for Scientific Research [16H01018, 26288047] Funding Source: KAKEN
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New iridium complexes having functional 8-quinolinolato ligands have been synthesized. By single-crystal X-ray analysis, it was revealed that these new complexes had coordinatively unsaturated structure (five-coordinate trivalent iridium: 16e(-) complex). Furthermore, one of the new complexes exhibited high catalytic activity for the dehydrogenative oxidation of various aromatic and aliphatic secondary alcohols in aqueous media to give the corresponding ketones in good to excellent yields.
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