Journal
CHEMICAL COMMUNICATIONS
Volume 53, Issue 37, Pages 5143-5146Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7cc01763d
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Funding
- Department of Science and Technology, India
- SERB
- DST [EMR/2014/001165]
- IIT Kanpur
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A highly diastereo- and enantioselective vinylogous Mukaiyama-Michael reaction of silyloxyfurans with alpha,beta-unsaturated 2-acyl imidazoles catalyzed by either chiral Sc(III) or Er(III) complexes of a pybox ligand has been reported. The enantioenriched gamma-butenolides formed in the reaction were further transformed into highly functionalized gamma-lactones found as important structural frameworks in a wide range of biologically active natural products.
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