Journal
SCIENTIFIC REPORTS
Volume 7, Issue -, Pages -Publisher
NATURE PUBLISHING GROUP
DOI: 10.1038/srep44697
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Funding
- National Basic Research Program of China [2013CB934800]
- National Natural Science Foundation of China (NSFC) [21573103, 21222302, 20903056]
- NSFC-Royal Society Joint Program [21661130149, 21111130201]
- Program for New Century Excellent Talents in University [NCET-10-0483]
- Fundamental Research Funds for the Central Universities [1124020512]
- National Science Fund for Talent Training in Basic Science [J1103310]
- Royal Society and Newton Fund for Royal Society - Newton Advanced Fellowship
- Priority Academic Program Development of Jiangsu Higher Education Institutions
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A simple and effective carbon-free strategy is carried out to prepare mixed molybdenum oxides as an advanced anode material for lithium-ion batteries. The new material shows a high specific capacity up to 930.6 mAh (.) g(-1), long cycle-life (> 200 cycles) and high rate capability. 1D and 2D solid-state NMR, as well as XRD data on lithiated sample (after discharge) show that the material is associated with both insertion/extraction and conversion reaction mechanisms for lithium storage. The well mixed molybdenum oxides at the microscale and the involvement of both mechanisms are considered as the key to the better electrochemical properties. The strategy can be applied to other transition metal oxides to enhance their performance as electrode materials.
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