Journal
RSC ADVANCES
Volume 7, Issue 35, Pages 21820-21826Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7ra01047h
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Funding
- Program to Solve Climate Changes of Korea (NRF) - Ministry of Science, ICT & Future Planning, Republic of Korea [NRF-2010-C1AAA001-2010-0029031]
- Climate Change Research Hub of KAIST [N01170224]
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Sodium ion batteries are a promising alternative to conventional lithium-ion batteries, mostly for large scale energy storage applications. In this paper, we report sodium vanadium oxy-fluorophosphate as a cathode material for sodium-ion batteries with 8.0 wt% reduced graphene oxide (rGO), synthesized via solid state reaction followed by a hydrothermal method. The newly reported Na3V2O2X(PO4)(2)F3-2X-rGO (NVOPF-rGO) composite with a hydrophilic carboxymethyl cellulose sodium (CMC-Na) binder shows enhanced rate performance and highly stable cyclability; it delivers a stable reversible capacity of 108 mA h g(-1) in a sodium half-cell, and it exhibits 98% capacity retention at a 0.1C rate over 250 cycles. Furthermore, the as-prepared NVOPF-rGO composite exhibits discharge capacities of 98 mA h g(-1) and 64 mA h g(-1) at 0.2C and 2C rates, respectively, in a full-cell configuration with a NaTi2(PO4) 3-MWCNT (NTP-M) anode for 1000 cycles.
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