Journal
RSC ADVANCES
Volume 7, Issue 39, Pages 24522-24536Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7ra03203j
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Funding
- Russian Science Foundation [15-03-30007]
- Russian Foundation for Basic Research (ERA.Net RUS Plus) [17-03-00131, 16-53-76007, SAS-MEM 254]
- German Academic Exchange Service [57130104]
- Russian Science Foundation [15-13-30007] Funding Source: Russian Science Foundation
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Amphiphilic narrow dispersed copolymers of acrylic acid and fluoroalkyl acrylates are synthesized via reversible addition-fragmentation chain transfer (RAFT) polymerization using dibenzyl trithiocarbonate in DMF solution. These copolymers and polyacrylic acid containing the trithiocarbonate group within the polymeric chain are used for the synthesis of triblock copolymers in organic, aqueous-organic or aqueous media by chain extension with n-butyl acrylate or its mixture with fluoroalkyl acrylates. Both dispersion polymerization and emulsifier-free emulsion polymerization lead to self-assembling of triblock copolymers in the core-shell particles; the former route provides the formation of microstructured polymer films with a percolated structure.
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