Journal
CHEMSUSCHEM
Volume 10, Issue 11, Pages 2380-2384Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201700630
Keywords
chromophores; electrochemistry; fluorinated polymers; phosphonic acid; water oxidation
Funding
- UNC EFRC Center for Solar Fuels, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001011]
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Here, the application of the fluorinated polymer [Dupont AF, a copolymer of 4,5-difluoro-2,2-bis(trifluoromethyl)-1,3-dioxole and tetrafluoroethylene] is described in stabilizing phosphonate-derivatized molecular assemblies on oxide electrodes. In the procedure, the polymer was dip-coated onto the surfaces of oxide electrodes with pre-bound, phosphonate-derivatized chromophores and assemblies, including assemblies for water oxidation. The results of the experiments showed a high degree of stabilization by the added polymer and a demonstration of its use in stabilizing surface-bound assemblies for water-oxidation catalysis.
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