Journal
CHEMICAL COMMUNICATIONS
Volume 53, Issue 51, Pages 6848-6851Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7cc03262e
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Funding
- National Natural Science Foundation of China [21622204, 21572186]
- Natural Science Foundation of Fujian Province for Distinguished Young Scholars [2015J06003]
- Qing Lan Project of Jiangsu Province
- Jiangsu University Foundation [13JDG059]
- NFFTBS [J1310024]
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A novel dual gold/photoredox-catalyzed bis-arylative cyclization of chiral homopropargyl sulfonamides with diazonium salts has been developed, allowing the facile synthesis of various enantioenriched 2,3-dihydropyrroles in generally moderate to good yields with excellent enantioselectivities under very mild conditions without using any strong oxidants. The reaction is proposed to undergo an Au-I/Au-III redox cycle promoted by visible-light photoredox catalysis.
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