Journal
CATALYSIS COMMUNICATIONS
Volume 98, Issue -, Pages 76-80Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.catcom.2017.05.009
Keywords
Work function; Soot combustion; Alkali tungsten bronzes; Alkali promotion
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The effect of bulk alkali (Li, Na, K, Cs) promotion on the tungsten(VI) oxide catalytic activity in soot oxidation was investigated. Catalyst oxidation and reduction susceptibility investigations have shown, that soot oxidation on the investigated catalysts operates through Mars van Krevelen mechanism. It has been also revealed, that increase in electrodonor properties (lowering the work function) of the A(X)WO(3) (A= Li, Na, K, Cs) catalysts results in enhancing the catalytic activity in soot oxidation with the promotional effect increasing in order: Cs < Na << K approximate to Li.
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