Journal
CATALYSIS SCIENCE & TECHNOLOGY
Volume 7, Issue 2, Pages 452-458Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cy02318e
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Funding
- National Natural Science Foundation of China [21503271]
- '1000 Talent Program' (The Recruitment Program of Global Experts)
- CAS/SAFEA International Partnership Program for Creative Research Teams
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Defects have a vital effect on the band structures and properties of semiconductor photocatalysts. Herein, we developed a one-step strategy to introduce defects in the framework of g-C3N4 by controllable copolymerization of melamine with a series of partially reactive end capped monomers. The capping molecules have great impacts on the properties of modified g-C3N4. The obtained defective g-C3N4 exhibits an increased surface area, improved charge carrier separation efficiency, and a narrowed band gap with a negative shift of the conduction band. Particularly, defect-rich CN-DPT shows 10 times improvement of visible light activity for hydrogen production compared with pristine g-C3N4.
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