Journal
ADVANCED ENERGY MATERIALS
Volume 8, Issue 10, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.201702369
Keywords
close-packed grains; low-angle grain boundaries; perovskite solar cells; preferred-orientation; pressure-induced crystallization
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Funding
- National Research Foundation of Korea (NRF) grant - Korean government [2016R1A2A1A05005216, 2017M3A7B4041987]
- Korea Institute of Energy Technology Evaluation and Planning (KETEP)
- Ministry of Trade, Industry & Energy (MOTIE) of the Republic of Korea [20163010012450]
- Global Frontier R&D Program of the Center for Multiscale Energy System - National Research Foundation under the Ministry of Science, ICT Future, Korea [NRF-2012M3A6A7054861]
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A general methodology is reported to create organic-inorganic hybrid metal halide perovskite films with enlarged and preferred-orientation grains. Simply pressing polyurethane stamps with hexagonal nanodot arrays on partially dried perovskite intermediate films can cause pressure-induced perovskite crystallization. This pressure-induced crystallization allows to prepare highly efficient perovskite solar cells (PSCs) because the preferred-orientation and enlarged grains with low-angle grain boundaries in the perovskite films exhibit suppressed nonradiative recombination. Consequently, the photovoltaic response is dramatically improved by the uniaxial compression in both inverted-planar PSCs and normal PSCs, leading to power conversion efficiencies of 19.16%.
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