Journal
ADVANCED SYNTHESIS & CATALYSIS
Volume 359, Issue 14, Pages 2358-2363Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201700178
Keywords
dehydrogenation; graphene oxide; heterogeneous catalysis; nitrogen heterocycles
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Funding
- National Natural Science Foundation of China [21402168]
- Scientific Research Foundation of Hunan Provincial Education Department [15B232]
- Hunan Collaborative Innovation Center of Chemical Engineering Technology
- Environmental Benignity
- Effective Resource Utilization
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Graphene oxide (GO) has been developed as an inexpensive, environmental friendly, metal-free carbocatalyst for the dehydrogenation of nitrogen heterocycles. Valuable compounds, such as quinoline, 3,4-dihydroisoquinoline, quinazoline, and indole derivatives, have been successfully used as substrates. The investigation of various oxygen-containing molecules with different conjugated systems indicated that both the oxygen-containing groups and large p-conjugated system in GO sheets are essential for this reaction.
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