Journal
CHEMSUSCHEM
Volume 10, Issue 14, Pages 2886-2890Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201700898
Keywords
carbon dioxide; cycloaddition; epoxides; homogeneous catalysis; rare earths
Funding
- Ministerio de Economia y Competitividad (MINECO) of Spain [CTQ2014-51912-REDC, CTQ2014-52899-R]
- Plan Propio de la Universidad de Castilla-La Mancha
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A new lanthanum heteroscorpionate complex has shown exceptional catalytic activity for the synthesis of cyclic carbonates from epoxides and carbon dioxide. This catalyst system also promotes the reaction of bio-based epoxides to give an important class of bis(cyclic carbonates) that can be further used for the production of bio-derived non-isocyanate polyurethanes. The catalytic process requires low catalyst loading and mild reaction conditions for the synthesis of a wide range of cyclic carbonates.
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